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4Fe-Cr-Ni合金裂解炉管1075 ℃渗碳行为研究
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合肥通用机械研究院有限公司 国家压力容器与管道安全工程技术研究中心 中国石化炉管质量检测检验与评估中心,安徽 合肥 230031

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TG132.3+3

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安徽省重点研发计划(202104a05020023);中国石油化工股份有限公司科技开发项目(36600000-23-ZC0607)


Carburizing Behavior of Four Kinds of Fe-Cr-Ni Alloy Cracking Furnace Tubes at 1075 ℃
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National Engineering & Technical Research Center on Pressure Vessels and Piping Safety, Sinopec Inspection and Assessment Center on Furnace Tube, Hefei General Machinery Research Institute Co., Ltd, Hefei 230031, China

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    摘要:

    为了分析Fe-Cr-Ni合金裂解炉管的抗渗碳性能,采用粒径为1.5~3 mm的固体渗碳剂对2种传统合金炉管25Cr35NiNb+MA(微合金)、35Cr45NiNb+MA和2种具有延长清焦周期效果的加铝合金炉管27Cr44Ni5W3Al+MA和29Cr44Ni4Al+MA开展了1075 ℃条件下50~200 h的渗碳试验研究。采用直读光谱仪、扫描电镜、X射线衍射仪、维氏硬度计等对渗碳试验后炉管进行成分、组织、性能分析,研究了渗碳动力学及组织转变规律。结果表明:4种材料渗碳层厚度均随渗碳时间延长而增加,1075 ℃、200 h渗碳试验后炉管渗碳层厚度分别约为2.0、1.8、1.0和0.7 mm,平均渗碳速度分别约为0.01、0.009、0.005和0.0035 mm/h,2种加铝合金炉管的抗渗碳性能优于传统炉管。27Cr44Ni5W3Al+MA炉管时效区组织为奥氏体+块状M23C6+鱼骨状M7C3,碳化物中“M”含Cr、W等元素,渗碳区块状M23C6转变为块状M7C3和WC,鱼骨状M7C3粗化。29Cr44Ni4Al+MA炉管时效区组织为奥氏体+块状M23C6+块状NbTiC,碳化物中“M”主要为Cr元素,渗碳区块状M23C6转变为块状M7C3,NbTiC由块状转变为颗粒状。2种加铝合金炉管内壁形成了致密稳定Al2O3膜,相比于传统炉管内壁Cr2O3膜,能够更有效地阻挡碳原子进入基体,提高抗渗碳性能。

    Abstract:

    To analyze the carburizing resistance of Fe-Cr-Ni alloy cracking furnace tube, solid carburizing agent with particle size of 1.5–3 mm was used to conduct carburizing test on two kinds of traditional furnace tubes (25Cr35NiNb+MA and 35Cr45NiNb+MA) as well as two kinds of aluminum-added alloy furnace tubes with prolonged coke cleaning period (27Cr44Ni5W3Al+MA and 29Cr44Ni4Al+MA). The test was carried out at 1075 ℃ for 50–200 h. The composition, microstructure and properties of the furnace tubes after carburizing test were analyzed by optical emission spectrometer, scanning electron microscope, X-ray diffractometer and Vickers hardness tester, and the carburizing kinetics and microstructure transformation rules were studied. The results show that the thickness of the carburized layer of four kinds of materials is increased with the prolongation of carburizing time. After carburizing at 1075 ℃ for 200 h, the thicknesses of the carburized layers of the furnace tubes are about 2.0, 1.8, 1.0 and 0.7 mm, and the average carburizing rates are about 0.01, 0.009, 0.005 and 0.0035 mm/h. The carburizing resistance of the two aluminum-added alloy tubes is better than that of the traditional tubes. The microstructure in the aged zone of 27Cr44Ni5W3Al+MA furnace tube is composed of austenite, blocky M23C6 and fishbone-like M7C3. The "M" in carbides contains elements such as Cr and W. In the carburized zone, blocky M23C6 is transformed into blocky M7C3 and WC, and fishbone-like M7C3 coarsens. The microstructure in the aged zone of 29Cr44Ni4Al+MA furnace tube is composed of austenite, blocky M23C6 and NbTiC. The "M" in carbides is mainly Cr element. In carburized zone, blocky M23C6 is transformed into blocky M7C3, and NbTiC changes from blocky to granular. The inner walls of two aluminum-added alloy furnace tubes form a dense and stable Al2O3 film. Compared with the Cr2O3 film on the inner walls of traditional furnace tubes, the Al2O3 film can more effectively block the penetration of carbon atoms into the substrate, thereby enhancing the anti-carburization performance.

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陈涛,刘春娇,吴志刚.4Fe-Cr-Ni合金裂解炉管1075 ℃渗碳行为研究[J].稀有金属材料与工程,2025,54(4):1034~1043.[Chen Tao, Liu Chunjiao, Wu Zhigang. Carburizing Behavior of Four Kinds of Fe-Cr-Ni Alloy Cracking Furnace Tubes at 1075 ℃[J]. Rare Metal Materials and Engineering,2025,54(4):1034~1043.]
DOI:10.12442/j. issn.1002-185X.20230779

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  • 收稿日期:2023-12-01
  • 最后修改日期:2024-01-09
  • 录用日期:2024-02-01
  • 在线发布日期: 2025-04-23
  • 出版日期: 2025-04-21