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A facile ball milling method for fabricating g-C3N4/MoS2 nanosheets heterojunction and its visible light photocatalytic performances
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School of Materials Science and Engineering,Chang’an University,Xi’an,School of Materials Science and Engineering,Chang’an University,Xi’an,School of Materials Science and Engineering,Chang’an University,Xi’an,School of Materials Science and Engineering,Chang’an University,Xi’an,School of Materials Science and Engineering,Chang’an University,Xi’an,School of Materials Science and Engineering,Chang’an University,Xi’an,School of Materials Science and Engineering,Chang’an University,Xi’an,School of Materials Science and Engineering,Chang’an University,Xi’an,School of Materials Science and Engineering,Chang’an University,Xi’an

Fund Project:

Natural Science Basis Research Plan in Shaanxi Province of China (2015JM2070), National Natural Science Foundation of China (51402024) and Fundamental Research Funds for the Central Universities ((300102318402).

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    Abstract:

    The g-C3N4/MoS2 nanosheets were prepared via a facile ball milling method. The composite photocatalysts were characterized by X-ray diffraction (XRD), high-resolution transmission electron microscopy (HRTEM), UV–vis diffuse reflectance spectroscopy (DRS) and photoluminescence (PL) spectroscopy. The results indicated that MoS2 nanosheets were successfully coupled into the g- C3N4 to form C3N4/ MoS2 heterojunction. The photocatalytic activities were evaluated by degradation of organic Rhodamine B (RhB) under visible light irradiation. The kinetic constant of RhB degradation with g-C3N4/MoS2 nanosheets-2 wt % heterojunction (0.0368 min?1) is about 4.3 as high as that of the bulk g-C3N4 (0.00840 min?1). The enhanced photocatalytic activities can be mainly ascribed to the efficient separation and transportation of photo-induced electron-hole pairs. The possible photocatalytic mechanism of composites was proposed according to the light trapping experiment.

    Reference
    1Hoffmann M R, Choi W Y, Bahnemann D W. Chem.Rev[J],1995, 95:69
    2Serpone N, Emeline AV. J. Phys. Chem. Lett[J], 2012,3:673
    3Linsebigler A L, Lu G, Yates J T. Chem.Rev[J],1995, 95:735
    4Singh S, Srivastava V C, Lo S L. Mater. Sci. Forum[J], 2016,85: 5105
    5Zhu HY, Jiang R, Xiao L et al. J.Hazard.Mater[J],2009,169: 933
    6Soltani N, Saion E, Hussein MZ et al. Int J Mol Sci[J],2012,131:175
    7Meenakshi G, Sivasamy A. Environ.Safe[J], 2017,135:243
    8Wang X C, Maeda K, Thomas A et al. Nat. Mater[J],2009,8:76 .
    9Mamba G, Mishra A K.Appl. Catal. B-Environ[J],2016,198:347
    10Yan S C, Li Z S, Zou Z G. Langmuir[J],2009,25:10397
    11Yuan X, Zhou C, Jin Y et al. J.Colloid . Interf. Sci[J], 2016,468: 211
    12Jiang D, Chen L, Zhu J et al. Dalton.T[J],2013,42:15726
    13Fang Z L, Rong H F, Zhou L Y et al. J.Mater.Sci[J], 2015,50:3057
    14Jiang D, Zhu J, Chen M et al. J.Colloid . Interf. Sci[J],2014,417:115.
    15Zhao J, Ji Z, Shen X et al. Ceram.Int[J],2015,41:5600.
    16Hu S W, Yang L W, Tian Y et al. Appl. Catal. B-Environ[J],2015,163:611
    17Peng W C, Li X Y. Catal. Commun[J], 2014,49: 63
    18Li Q, Zhang N, Yang Y, et al. Langmuir[J], 2014,30:8965
    19Tian Y, Ge L, Wang K et al. Mater. Charact[J],2014,87:70
    20Zhang W, Xiao X, Li Y et al. Appl. Surf. Sci[J],2016,389:496
    21Ye L, Wang D, Chen S et al. ACS. Appl. Mater. Inter[J], 2016,8:5280
    22Wang J, Guan Z, Huang J et al. J.Mater. Chem. A[J], 2014,2:7960
    23Zhao H, Dong Y, Jiang P et al. J.Mater.Chem.A[J], 2015,3:7375
    24Ge L, Han C, Xiao X et al. Int.J.Hydrogen Energ[J], 2013,38: 6960
    25Li J, Liu E Z, Ma Y N et al.Appl. Surf. Sci[J],2016,364:694
    26Zhao H, Dong Y, Jiang P et al. J.Mater.Chem.A[J], 2015,3:7375
    27Lu X, Jin Y, Zhang X et al. Dalton. T[J],2016,45:15406
    28Hou Y, Wen Z, Cui S et al. Adv. Mater[J],2013,25:6291
    29Yao Y, Lin Z, Li Z et al. J.Mater.Chem[J], 2012,22:13494
    30Shi W, Guo F, Chen J et al. J. Alloy. Compd[J], 2014,612:143
    31Liu W, Wang M, Xu C et al.J. Mol. Catal. A: chem[J], 2013. 368-369:9
    32Liu L, Qi Y, Yang J et al. Appl. Surf. Sci[J],2015,358:319
    33Miao H, Zhang G, Hu X et al. J. Alloy. Compd[J],2017,690:669.
    34Yan S C, Lv S B, Li Z S et al. Dalton.T[J], 2010,39:1488
    35Ellis J K, Lucero M J, Scuseria GE. Appl. Phys. Lett[J], 2011,99:261908
    36Jo W K, Lee J Y, Sagaya N C. Chem. Eng. J[J],2016,289:306
    37Chen X, Tan P, Zhou B et al. J. Alloys.Compd[J], 2015,647:456
    38Lv H, Ji G, Yang Zet al. J. Colloid Interface Sci[J],2015,450:381
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[Yan Xin, Gao Qiang, Hui Xiaoyan, Yan Congxiang, AiTao, WangZhenjun, Sun Guodong, Su Xinghua, Zhao Peng. A facile ball milling method for fabricating g-C3N4/MoS2 nanosheets heterojunction and its visible light photocatalytic performances[J]. Rare Metal Materials and Engineering,2018,47(10):3015~3020.]
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History
  • Received:March 17,2017
  • Revised:August 15,2018
  • Adopted:April 13,2017
  • Online: November 08,2018